Influence of the preparation method in the metal-support interaction and reducibility of Ni-Mg-Al based catalysts for methane steam reforming

Description

Ni-Mg-Al based catalysts were prepared using different preparation methods (impregnation, impregnation-coprecipitation and coprecipitation) and tested in steam reforming of methane. The differences observed in catalytic activity were directly correlated to the physicochemical properties and the different degree of Ni-Mg-Al interaction. The reducibility results showed that the catalyst prepared by the impregnation-coprecipitation method presented the most optimal metal-support interaction to reduce the NiO preserving the Ni0 particles highly dispersed on the support surface. These results demonstrate that the structure and catalytic performance of Ni-Mg-Al based catalysts can be tuned by controlling the metal-support interaction through of the preparation method.

Abstract

Ministerio de Economía y Competitividad ENE2015-66975-C3-2-R

Abstract

Fondo Europeo de Desarrollo Regional (FEDER) IJCI-2015-26348, RYC-2013-12437

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